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In the special case of the condensed-ring aromatic hydrocar­ bons, the principal anisotropy is with respect to the axis normal to the ring plane; since all C-H axes are in this plane, the correlation times should be similar. The nuclear Overhauser enhancement for different carbon atoms with similar proton environments may differ, however, if the orientations of the C-H vectors differ relative to the rotational diffusion tensor. Thus, Eq. 12] may be misleading and their more general form must be applied for the latter situations.

50. W. A. McFarlane in "Annual Review of NMR Spectroscopy" (E. F. ), Vol. 1, p. 135. Academic Press, New York, 1968. 51. R. A. Hoffman and S. Forsen in "Progress in Nuclear Magnetic Resonance Spectroscopy" (J. W. Emsley, J. Feeney and L. H. ), Vol. 1, p. 15. Pergamon Press, London, 1966. 52. H. Spiesecke and W. G. Schneider, J. Chem. Phys. 35, 722 (1961). 53. R. Freeman, J. Chem. Phys. 40, 3571 (1964). 54. A. J. Jones and D. M. Grant, Chem. , 72, in press (1972). 55. P. Laszlo in "Progress in Nuclear Magnetic Resonance Spectroscopy" (J.

Rev. 92, 411 (1953). 20. K. F. Kuhlmann and D. M. Grant, J. Am. Chem. Soc. 90, 7355 (1968). 21. I. Solomon, Phys. Rev. 99, 559 (1955). 22. A. J. Jones, D. M. Grant and K. F. Kuhlmann, J. Am. Chem. Soc. 91, 5013 (1969). 23. K. F. Kuhlmann, D. M. Grant and R. K. Harris, J. Chem. Phys. 52, 3439 (1970). 23a. G. La Mar, / . Am. Chem. Soc. 93, 1040 (1971). 23b. D. F. S. Natusch, J. Am. Chem. Soc. 93, 2566 (1971). References 51 24. R. A. Dwek, J. G. Kenworthy, D. F. S. Natusch, R. E. Richards and D. J.

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